Among my favorite SEGA CD games:
Earthworm Jim: Special Edition
Sonic CD (duh!)
Battlecorps
Ecco: The Tides of Time
Sylpheed
Pitfall: The Mayan Adventure
If you like a REALLY tough platformer, Shadow of the Beast II is available for the SEGA CD.
I never got into "FMV" games, but many people enjoy them. The most popular is probably Sewer Shark.
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